Convergent beam electron holography for analysis of van der Waals heterostructures

T. Latychevskaia, Colin Woods, Yibo Wang, Matthew Holwill, Eric Prestat, Sarah Haigh, Konstantin Novoselov

    Research output: Contribution to journalArticlepeer-review

    Abstract

    Van der Waals heterostructures, which explore the synergetic properties of two-dimensional (2D) materials when assembled into three-dimensional stacks, have already brought to life a number of exciting new phenomena and novel electronic devices. Still, the interaction between the layers in such assembly, possible surface reconstruction, intrinsic and extrinsic defects are very difficult to characterise by any method, because of the single-atomic nature of the crystals involved. Here we present a convergent beam electron holographic technique which allows imaging of the stacking order in such heterostructures. Based on the interference of electron waves scattered on different crystals in the stack, this approach allows one to reconstruct the relative rotation, stretching, out-of-plane corrugation of the layers with atomic precision. Being holographic in nature, our approach allows extraction of quantitative information about the three-dimensional structure of the typical defects from a single image covering thousands of square nanometres. Furthermore, qualitative information about the defects in the stack can be extracted from the convergent diffraction patterns even without reconstruction – simply by comparing the patterns in different diffraction spots. We expect that convergent beam electron holography will be widely used to study the properties of van der Waals heterostructures.
    Original languageEnglish
    JournalProceedings of the National Academy of Sciences
    Early online date3 Jul 2018
    DOIs
    Publication statusPublished - 3 Jul 2018

    Keywords

    • Graphene
    • Two-dimensional Materials
    • van der Waals Structures
    • Electron Holography
    • Convergent Beam Electron Diffraction

    Research Beacons, Institutes and Platforms

    • National Graphene Institute

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