Ethanol Steam Reforming for Hydrogen Production Over Hierarchical Macroporous Mesoporous SBA-15 Supported Nickel Nanoparticles

Christopher M. A. Parlett; Lee J. Durndell; Mark A. Isaacs; Xiaotong Liu; Chunfei Wu

doi:10.1007/s11244-020-01265-4

Ethanol Steam Reforming for Hydrogen Production Over Hierarchical Macroporous Mesoporous SBA-15 Supported Nickel Nanoparticles

Christopher M. A. Parlett, Lee J. Durndell, Mark A. Isaacs, Xiaotong Liu, Chunfei Wu

CE - Academic & Research

Research output: Contribution to journal › Article › peer-review

Abstract

The influence of complementary macropores, present in hierarchical macroporous mesoporous SBA-15, on the performance of supported Ni nanoparticles for ethanol steam reforming has been investigated. The increased open nature of the architecture, afforded through the incorporation of the secondary macropore network, enables superior metal dispersion. This, in turn, enhances catalytic hydrogen production performance through the generation of a greater density of active sites.

Original language	English
Pages (from-to)	403-412
Number of pages	10
Journal	Topics in Catalysis
Volume	63
Issue number	3-4
Early online date	6 May 2020
DOIs	https://doi.org/10.1007/s11244-020-01265-4
Publication status	Published - 1 Jul 2020

Keywords

Ethanol steam reforming
Hierarchical porous materials
Hydrogen production
Macroporous mesoporous SBA-15
Nanoparticles
Nickel

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10.1007/s11244-020-01265-4Licence: CC BY

http://link.springer.com/10.1007/s11244-020-01265-4

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title = "Ethanol Steam Reforming for Hydrogen Production Over Hierarchical Macroporous Mesoporous SBA-15 Supported Nickel Nanoparticles",

abstract = "The influence of complementary macropores, present in hierarchical macroporous mesoporous SBA-15, on the performance of supported Ni nanoparticles for ethanol steam reforming has been investigated. The increased open nature of the architecture, afforded through the incorporation of the secondary macropore network, enables superior metal dispersion. This, in turn, enhances catalytic hydrogen production performance through the generation of a greater density of active sites.",

keywords = "Ethanol steam reforming, Hierarchical porous materials, Hydrogen production, Macroporous mesoporous SBA-15, Nanoparticles, Nickel",

author = "Parlett, {Christopher M. A.} and Durndell, {Lee J.} and Isaacs, {Mark A.} and Xiaotong Liu and Chunfei Wu",

note = "Funding Information: XPS data analysis was performed at the EPSRC National Facility for XPS ({\textquoteleft}HarwellXPS{\textquoteright}), operated by Cardiff University and UCL, under contract No. PR16195. The authors declare that they have no conflict of interest. Publisher Copyright: {\textcopyright} 2020, The Author(s).",

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AU - Isaacs, Mark A.

AU - Liu, Xiaotong

AU - Wu, Chunfei

N1 - Funding Information: XPS data analysis was performed at the EPSRC National Facility for XPS (‘HarwellXPS’), operated by Cardiff University and UCL, under contract No. PR16195. The authors declare that they have no conflict of interest. Publisher Copyright: © 2020, The Author(s).

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N2 - The influence of complementary macropores, present in hierarchical macroporous mesoporous SBA-15, on the performance of supported Ni nanoparticles for ethanol steam reforming has been investigated. The increased open nature of the architecture, afforded through the incorporation of the secondary macropore network, enables superior metal dispersion. This, in turn, enhances catalytic hydrogen production performance through the generation of a greater density of active sites.

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KW - Hydrogen production

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KW - Nickel

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Ethanol Steam Reforming for Hydrogen Production Over Hierarchical Macroporous Mesoporous SBA-15 Supported Nickel Nanoparticles

Abstract

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UoMaH: The University of Manchester at Harwell

Cite this

Ethanol Steam Reforming for Hydrogen Production Over Hierarchical Macroporous Mesoporous SBA-15 Supported Nickel Nanoparticles

Abstract

Keywords

Access to Document

Other files and links

Fingerprint

Projects

UoMaH: The University of Manchester at Harwell

Cite this