Abstract
We study the low-energy surface electronic structure of the transition-metal dichalcogenide superconductor
PdTe
2
by spin- and angle-resolved photoemission, scanning tunneling microscopy, and density-functional theory-based supercell calculations. Comparing
PdTe
2
with its sister compound
PtSe
2
, we demonstrate how enhanced interlayer hopping in the Te-based material drives a band inversion within the antibonding
p
-orbital manifold well above the Fermi level. We show how this mediates spin-polarized topological surface states which form rich multivalley Fermi surfaces with complex spin textures. Scanning tunneling spectroscopy reveals type-II superconductivity at the surface, and moreover shows no evidence for an unconventional component of its superconducting order parameter, despite the presence of topological surface states.
PdTe
2
by spin- and angle-resolved photoemission, scanning tunneling microscopy, and density-functional theory-based supercell calculations. Comparing
PdTe
2
with its sister compound
PtSe
2
, we demonstrate how enhanced interlayer hopping in the Te-based material drives a band inversion within the antibonding
p
-orbital manifold well above the Fermi level. We show how this mediates spin-polarized topological surface states which form rich multivalley Fermi surfaces with complex spin textures. Scanning tunneling spectroscopy reveals type-II superconductivity at the surface, and moreover shows no evidence for an unconventional component of its superconducting order parameter, despite the presence of topological surface states.
Original language | English |
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Journal | Physical Review Letters |
DOIs | |
Publication status | Published - 9 Apr 2018 |