In-situ X-ray studies of clean catalytic technologies

Adam F. Lee; Christine V. Ellis; Mark A. Newton; Christopher M. Parlett; Karen Wilson

doi:10.1557/opl.2011.1170

In-situ X-ray studies of clean catalytic technologies

Adam F. Lee^*, Christine V. Ellis, Mark A. Newton, Christopher M. Parlett, Karen Wilson

^*Corresponding author for this work

Research output: Chapter in Book/Conference proceeding › Conference contribution › peer-review

Abstract

The rational design of new heterogeneous catalysts for clean chemical technologies can be accelerated by molecular level insight into surface chemical processes. In-situ methodologies, able to provide time-resolved and/or pressure dependent information on the evolution of reacting adsorbed layers over catalytically relevant surfaces, are therefore of especial interest. Here we discuss the application of in-situ XPS and in-situ, synchronous DRIFTS/MS/XAS methodologies to elucidate the active site in Pd-catalyzed, selective aerobic oxidation of allylic alcohols.

Original language	English
Title of host publication	Surfaces and Nanomaterials for Catalysis through In-Situ or Ex-Situ Studies
Pages	32-37
Number of pages	6
Volume	1351
DOIs	https://doi.org/10.1557/opl.2011.1170
Publication status	Published - 1 Dec 2011
Event	2011 MRS Spring Meeting - San Francisco, CA, United States Duration: 25 Apr 2011 → 29 Apr 2011

Publication series

Name	Materials Research Society Symposium Proceedings
Publisher	Cambridge University Press
Volume	1351
ISSN (Print)	0272-9172

Conference

Conference	2011 MRS Spring Meeting
Country/Territory	United States
City	San Francisco, CA
Period	25/04/11 → 29/04/11

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10.1557/opl.2011.1170

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title = "In-situ X-ray studies of clean catalytic technologies",

abstract = "The rational design of new heterogeneous catalysts for clean chemical technologies can be accelerated by molecular level insight into surface chemical processes. In-situ methodologies, able to provide time-resolved and/or pressure dependent information on the evolution of reacting adsorbed layers over catalytically relevant surfaces, are therefore of especial interest. Here we discuss the application of in-situ XPS and in-situ, synchronous DRIFTS/MS/XAS methodologies to elucidate the active site in Pd-catalyzed, selective aerobic oxidation of allylic alcohols.",

author = "Lee, \{Adam F.\} and Ellis, \{Christine V.\} and Newton, \{Mark A.\} and Parlett, \{Christopher M.\} and Karen Wilson",

year = "2011",

month = dec,

day = "1",

doi = "10.1557/opl.2011.1170",

language = "English",

isbn = "9781618395542",

volume = "1351",

series = "Materials Research Society Symposium Proceedings ",

publisher = "Cambridge University Press",

pages = "32--37",

booktitle = "Surfaces and Nanomaterials for Catalysis through In-Situ or Ex-Situ Studies",

note = "2011 MRS Spring Meeting ; Conference date: 25-04-2011 Through 29-04-2011",

}

Lee, AF, Ellis, CV, Newton, MA, Parlett, CM & Wilson, K 2011, In-situ X-ray studies of clean catalytic technologies. in Surfaces and Nanomaterials for Catalysis through In-Situ or Ex-Situ Studies. vol. 1351, Materials Research Society Symposium Proceedings , vol. 1351, pp. 32-37, 2011 MRS Spring Meeting, San Francisco, CA, United States, 25/04/11. https://doi.org/10.1557/opl.2011.1170

In-situ X-ray studies of clean catalytic technologies. / Lee, Adam F.; Ellis, Christine V.; Newton, Mark A. et al.
Surfaces and Nanomaterials for Catalysis through In-Situ or Ex-Situ Studies. Vol. 1351 2011. p. 32-37 (Materials Research Society Symposium Proceedings ; Vol. 1351).

Research output: Chapter in Book/Conference proceeding › Conference contribution › peer-review

TY - GEN

T1 - In-situ X-ray studies of clean catalytic technologies

AU - Lee, Adam F.

AU - Ellis, Christine V.

AU - Newton, Mark A.

AU - Parlett, Christopher M.

AU - Wilson, Karen

PY - 2011/12/1

Y1 - 2011/12/1

N2 - The rational design of new heterogeneous catalysts for clean chemical technologies can be accelerated by molecular level insight into surface chemical processes. In-situ methodologies, able to provide time-resolved and/or pressure dependent information on the evolution of reacting adsorbed layers over catalytically relevant surfaces, are therefore of especial interest. Here we discuss the application of in-situ XPS and in-situ, synchronous DRIFTS/MS/XAS methodologies to elucidate the active site in Pd-catalyzed, selective aerobic oxidation of allylic alcohols.

AB - The rational design of new heterogeneous catalysts for clean chemical technologies can be accelerated by molecular level insight into surface chemical processes. In-situ methodologies, able to provide time-resolved and/or pressure dependent information on the evolution of reacting adsorbed layers over catalytically relevant surfaces, are therefore of especial interest. Here we discuss the application of in-situ XPS and in-situ, synchronous DRIFTS/MS/XAS methodologies to elucidate the active site in Pd-catalyzed, selective aerobic oxidation of allylic alcohols.

UR - https://www.scopus.com/pages/publications/84860203193

U2 - 10.1557/opl.2011.1170

DO - 10.1557/opl.2011.1170

M3 - Conference contribution

AN - SCOPUS:84860203193

SN - 9781618395542

VL - 1351

T3 - Materials Research Society Symposium Proceedings

SP - 32

EP - 37

BT - Surfaces and Nanomaterials for Catalysis through In-Situ or Ex-Situ Studies

T2 - 2011 MRS Spring Meeting

Y2 - 25 April 2011 through 29 April 2011

ER -

In-situ X-ray studies of clean catalytic technologies

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