TY - JOUR
T1 - Pore-scale simulation of multiphase flow and reactive transport processes involved in geologic carbon sequestration
AU - Wang, Wendong
AU - Xie, Qiuheng
AU - An, Senyou
AU - Bakhshian, Sahar
AU - Kang, Qinjun
AU - Wang, Han
AU - Xu, Xinyue
AU - Su, Yuliang
AU - Cai, Jianchao
AU - Yuan, Bin
N1 - Publisher Copyright:
© 2023 Elsevier B.V.
PY - 2023/12/1
Y1 - 2023/12/1
N2 - Multiphase flow and reactive transport are two essential physicochemical processes that govern the effectiveness of geological carbon sequestration (GCS). The interaction and feedback among different phases and components during intricate physicochemical processes hold great significance in understanding CO
2 sequestration. Pore-scale simulations can account for multiphase flow and reactive transport processes in porous media and obtain spatial distributions of parameters (density, velocity, concentration, etc.) in the pore space as well as their temporal evolutions. This proves especially valuable considering that experiments can be hindered by constraints in spatial and temporal resolution. The comprehensive insights garnered from pore-scale research can be leveraged for continuum modeling using the representative elementary volume (REV) concept. In this contribution, four sequential mechanisms of CO
2-brine-rock interaction in three zones delineated by CO
2 saturation are elaborated to elucidate complicated physicochemical processes involved in GCS, which are followed by general descriptions of mathematical equations and pore-scale numerical methods. In addition, as interested and commonly encountered processes, leakage risks during GCS and CO
2-enhanced oil recovery (CO
2-EOR) processes are presented. The existing challenges and future directions are discussed for both the performance of the pore-scale models and the current gaps in the field of GCS. We expect that this review will prove beneficial for researchers interested in pore-scale simulations, GCS, and related disciplines.
AB - Multiphase flow and reactive transport are two essential physicochemical processes that govern the effectiveness of geological carbon sequestration (GCS). The interaction and feedback among different phases and components during intricate physicochemical processes hold great significance in understanding CO
2 sequestration. Pore-scale simulations can account for multiphase flow and reactive transport processes in porous media and obtain spatial distributions of parameters (density, velocity, concentration, etc.) in the pore space as well as their temporal evolutions. This proves especially valuable considering that experiments can be hindered by constraints in spatial and temporal resolution. The comprehensive insights garnered from pore-scale research can be leveraged for continuum modeling using the representative elementary volume (REV) concept. In this contribution, four sequential mechanisms of CO
2-brine-rock interaction in three zones delineated by CO
2 saturation are elaborated to elucidate complicated physicochemical processes involved in GCS, which are followed by general descriptions of mathematical equations and pore-scale numerical methods. In addition, as interested and commonly encountered processes, leakage risks during GCS and CO
2-enhanced oil recovery (CO
2-EOR) processes are presented. The existing challenges and future directions are discussed for both the performance of the pore-scale models and the current gaps in the field of GCS. We expect that this review will prove beneficial for researchers interested in pore-scale simulations, GCS, and related disciplines.
KW - Geological carbon sequestration
KW - Multiphase flow
KW - Pore-scale simulation
KW - Reactive transport
UR - http://www.scopus.com/inward/record.url?scp=85175418771&partnerID=8YFLogxK
UR - https://www.mendeley.com/catalogue/f3ea2372-f4d8-35d8-9e46-8f2f7c1e6fe8/
U2 - 10.1016/j.earscirev.2023.104602
DO - 10.1016/j.earscirev.2023.104602
M3 - Article
SN - 0012-8252
VL - 247
JO - Earth-Science Reviews
JF - Earth-Science Reviews
M1 - 104602
ER -
