Abstract
We report the results from an operando XRD-CT study of a working catalytic membrane reactor for the oxidative coupling of methane. These results reveal the importance of the evolving solid state chemistry during catalytic reaction, particularly the chemical interaction between the catalyst and the oxygen transport membrane.
Original language | English |
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Pages (from-to) | 12752-12755 |
Number of pages | 4 |
Journal | Chemical Communications |
Volume | 51 |
Issue number | 64 |
DOIs | |
Publication status | Published - 2015 |
Keywords
- x-ray-diffraction
- hollow-fiber membranes
- active phase evolution
- computed-tomography
- oxygen permeation
- natural-gas
- ceramic membrane
- oxide membranes
- ethylene
- conversion